Author, as appears in the article.: Aktas, Ece; Phung, Nga; Koebler, Hans; Gonzalez, Dora A.; Mendez, Maria; Kafedjiska, Ivona; Turren-Cruz, Silver-Hamill; Wenisch, Robert; Lauermann, Iver; Abate, Antonio; Palomares, Emilio;
Department: Química Física i Inorgànica
URV's Author/s: Aktas, Ece / González Ruiz, Dora Alejandra / MÉNDEZ MÁLAGA, MARIA
Keywords: Tio2 Sensitizers Performance Monolayers Light Layer Hysteresis Hole transporting materials Degradation
Abstract: Current perovskite solar cell efficiency is close to silicon's record values. Yet, the roadblock for industrialization of this technology is its stability. The stability of the solar cell not only depends on the stability of the perovskite material itself but also notably on its contact layers and their interface with the perovskite, which plays a paramount role. This study rationalizes the design of new molecules to form self-assembled monolayers as a hole-selective contact. The new molecules increased the stability of the perovskite solar cells to maintain 80% of their initial PCE of 21% for 250 h at 85 degrees C under 1 sun illumination. The excellent charge collection properties as well as perovskite passivation effect enable the highly stable and efficient devices to demonstrate the vast potential of this new type of contact in photovoltaic application.
Thematic Areas: Renewable energy, sustainability and the environment Química Pollution Nuclear energy and engineering Materiais Environmental sciences Environmental chemistry Engineering, chemical Engenharias iv Engenharias ii Engenharias i Energy & fuels Chemistry, multidisciplinary Biotecnología Astronomia / física
licence for use: https://creativecommons.org/licenses/by/3.0/es/
Author identifier: 0000-0002-4381-4456
Author's mail: doraalejandra.gonzalez@estudiants.urv.cat
Record's date: 2024-07-27
Papper version: info:eu-repo/semantics/acceptedVersion
Link to the original source: https://www.researchgate.net/publication/351784150_Understanding_the_perovskiteself-assembled_selective_contact_interface_for_ultra-stable_and_highly_efficient_p-i-n_perovskite_solar_cells
Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
Papper original source: Energy & Environmental Science. 14 (7): 3976-3985
APA: Aktas, Ece; Phung, Nga; Koebler, Hans; Gonzalez, Dora A.; Mendez, Maria; Kafedjiska, Ivona; Turren-Cruz, Silver-Hamill; Wenisch, Robert; Lauermann, Iv (2021). Understanding the perovskite/self-assembled selective contact interface for ultra-stable and highly efficient p-i-n perovskite solar cells. Energy & Environmental Science, 14(7), 3976-3985. DOI: 10.1039/d0ee03807e
Article's DOI: 10.1039/d0ee03807e
Entity: Universitat Rovira i Virgili
Journal publication year: 2021
Publication Type: Journal Publications