Articles producció científica> Enginyeria Química

Monodisperse droplets and particles by efficient neutralization of electrosprays

  • Datos identificativos

    Identificador: imarina:9242301
  • Autores:

    Carrasco-Munoz A
    Barbero-Colmenar E
    Bodnár E
    Grifoll J
    Rosell-Llompart J
  • Otros:

    Autor según el artículo: Carrasco-Munoz A; Barbero-Colmenar E; Bodnár E; Grifoll J; Rosell-Llompart J
    Departamento: Enginyeria Química
    Autor/es de la URV: GRIFOLL TAVERNA, JORDI / Rosell Llompart, Joan
    Palabras clave: charge reduction corona discharge coupling electrospray curcumin droplet to particle drug dynamic atomization electrical charge electrohydrodynamic atomization electrospray gas phase ions generation polymer microparticles polymer nanoparticles polymer particles spray Cone-jet mode Corona discharge Corona discharges Curcumin Droplet to particle Droplets Drops Electric corona Electrical charge Electrical charges Electrodes Electrohydrodynamic atomization Electrohydrodynamics Electrospray Electrosprays Extraction Gas phase ions Ion sources Nanoparticles Polymer microparticles Polymer nanoparticles Ring electrodes Size distribution
    Resumen: We present a new approach for micro- and nanoparticle production by in-situ charge reduction of electrospray droplets, which prevents their Coulombic instabilities and allow the efficient transport (extraction) of the particles. A unipolar ion source based on corona discharge generates a controllable ion flux of opposite polarity to the electrospray. The ions are introduced axially into the spray, while the Taylor cone is screened from the ions by an extractor ring electrode. Efficient and steady droplet discharge and extraction through an orthogonal aerosol-extraction tube was attained when the inlet of the tube was near the spray emission and the ring electrode, resulting in dramatic changes in droplets’ trajectories. The best extraction conditions (highest filter collections) were associated with the best discharging (lowest residual electrical charge) and the most globular particles. The size distributions on the particles collected on the filters were monomodal and homogeneous, with small relative standard deviations (as small as 10.6%). The use of corona ions significantly expands the range of polymer concentrations over which globular particles with monomodal size distribution can be made by electrospray. © 2021 Elsevier Ltd
    Áreas temáticas: Atmospheric science Engineering, chemical Engineering, mechanical Environmental chemistry Environmental engineering Environmental sciences Fluid flow and transfer processes General materials science Materials science (miscellaneous) Mechanical engineering Meteorology & atmospheric sciences Pollution Química
    Acceso a la licencia de uso: https://creativecommons.org/licenses/by/3.0/es/
    Direcció de correo del autor: joan.rosell@urv.cat
    Identificador del autor: 0000-0002-5288-9150
    Fecha de alta del registro: 2023-02-19
    Versión del articulo depositado: info:eu-repo/semantics/publishedVersion
    Enlace a la fuente original: https://www.sciencedirect.com/science/article/pii/S0021850221006352
    Referencia al articulo segun fuente origial: Journal Of Aerosol Science. 160
    Referencia de l'ítem segons les normes APA: Carrasco-Munoz A; Barbero-Colmenar E; Bodnár E; Grifoll J; Rosell-Llompart J (2022). Monodisperse droplets and particles by efficient neutralization of electrosprays. Journal Of Aerosol Science, 160(), -. DOI: 10.1016/j.jaerosci.2021.105909
    URL Documento de licencia: http://repositori.urv.cat/ca/proteccio-de-dades/
    DOI del artículo: 10.1016/j.jaerosci.2021.105909
    Entidad: Universitat Rovira i Virgili
    Año de publicación de la revista: 2022
    Tipo de publicación: Journal Publications
  • Palabras clave:

    Atmospheric Science,Engineering, Chemical,Engineering, Mechanical,Environmental Chemistry,Environmental Engineering,Environmental Sciences,Fluid Flow and Transfer Processes,Materials Science (Miscellaneous),Mechanical Engineering,Meteorology & Atmospheric Sciences,Pollution
    charge reduction
    corona discharge
    coupling electrospray
    curcumin
    droplet to particle
    drug
    dynamic atomization
    electrical charge
    electrohydrodynamic atomization
    electrospray
    gas phase ions
    generation
    polymer microparticles
    polymer nanoparticles
    polymer particles
    spray
    Cone-jet mode
    Corona discharge
    Corona discharges
    Curcumin
    Droplet to particle
    Droplets
    Drops
    Electric corona
    Electrical charge
    Electrical charges
    Electrodes
    Electrohydrodynamic atomization
    Electrohydrodynamics
    Electrospray
    Electrosprays
    Extraction
    Gas phase ions
    Ion sources
    Nanoparticles
    Polymer microparticles
    Polymer nanoparticles
    Ring electrodes
    Size distribution
    Atmospheric science
    Engineering, chemical
    Engineering, mechanical
    Environmental chemistry
    Environmental engineering
    Environmental sciences
    Fluid flow and transfer processes
    General materials science
    Materials science (miscellaneous)
    Mechanical engineering
    Meteorology & atmospheric sciences
    Pollution
    Química
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