Articles producció científica> Química Física i Inorgànica

Crystal growth, spectroscopy and first laser operation of a novel disordered tetragonal Tm:Na2La4(WO4)7tungstate crystal

  • Dades identificatives

    Identificador: imarina:3996506
    Autors:
    Zhang, LizhenSun, ShijiaLin, ZhoubinLin, HaifengZhang, GeMateos, XavierMaria Serres, JosepAguilo, MagdalenaDiaz, FrancescLoiko, PavelWang, YichengGriebner, UwePetrov, ValentinVilejshikova, ElenaChen, Weidong
    Resum:
    © 2018 Elsevier B.V. Tm3+:Na2La4(WO4)7, a disordered tetragonal scheelite-type tungstate crystal, is grown by the Czochralski method. The polarized absorption, stimulated-emission and gain cross-section spectra are determined. The maximum σSEis 1.62 × 10–20cm2at 1788.6 nm for σ-polarization. The Judd-Ofelt parameters for Tm3+are Ω2= 10.321, Ω4= 0.183 and Ω6= 2.122 [10–20cm2]. The radiative lifetime of the3F4state is 1.63 ms. Raman spectroscopy reveals a maximum phonon energy of 923 cm−1. Laser operation under diode-pumping is achieved with both a-cut and c-cut Tm:Na2La4(WO4)7crystals, reaching a maximum output power for the a-cut of 715 mW at ~ 1937 nm with a slope efficiency of 34%. Microchip laser operation using the c-cut crystal yields a slope efficiency of 41%. The Tm:Na2La4(WO4)7crystal is promising for mode-locked lasers due to its broadband emission.
  • Altres:

    Autor segons l'article: Zhang, Lizhen; Sun, Shijia; Lin, Zhoubin; Lin, Haifeng; Zhang, Ge; Mateos, Xavier; Maria Serres, Josep; Aguilo, Magdalena; Diaz, Francesc; Loiko, Pavel; Wang, Yicheng; Griebner, Uwe; Petrov, Valentin; Vilejshikova, Elena; Chen, Weidong
    Departament: Química Física i Inorgànica
    Autor/s de la URV: Aguiló Díaz, Magdalena / Díaz González, Francisco Manuel / Mateos Ferré, Xavier / Serres Serres, Josep Maria
    Paraules clau: Thulium ions Seven tungstates Luminescence Laser operation Judd-ofelt theory Absorption
    Resum: © 2018 Elsevier B.V. Tm3+:Na2La4(WO4)7, a disordered tetragonal scheelite-type tungstate crystal, is grown by the Czochralski method. The polarized absorption, stimulated-emission and gain cross-section spectra are determined. The maximum σSEis 1.62 × 10–20cm2at 1788.6 nm for σ-polarization. The Judd-Ofelt parameters for Tm3+are Ω2= 10.321, Ω4= 0.183 and Ω6= 2.122 [10–20cm2]. The radiative lifetime of the3F4state is 1.63 ms. Raman spectroscopy reveals a maximum phonon energy of 923 cm−1. Laser operation under diode-pumping is achieved with both a-cut and c-cut Tm:Na2La4(WO4)7crystals, reaching a maximum output power for the a-cut of 715 mW at ~ 1937 nm with a slope efficiency of 34%. Microchip laser operation using the c-cut crystal yields a slope efficiency of 41%. The Tm:Na2La4(WO4)7crystal is promising for mode-locked lasers due to its broadband emission.
    Àrees temàtiques: Química Optics Odontología Medicina ii Medicina i Materiais Interdisciplinar General chemistry Farmacia Ensino Engenharias iv Engenharias iii Engenharias ii Condensed matter physics Ciências biológicas ii Ciências biológicas i Ciências ambientais Ciência de alimentos Chemistry (miscellaneous) Chemistry (all) Biotecnología Biophysics Biochemistry Atomic and molecular physics, and optics Astronomia / física
    Accès a la llicència d'ús: https://creativecommons.org/licenses/by/3.0/es/
    ISSN: 00222313
    Adreça de correu electrònic de l'autor: josepmaria.serres@urv.cat magdalena.aguilo@urv.cat xavier.mateos@urv.cat f.diaz@urv.cat
    Identificador de l'autor: 0000-0002-4299-538X 0000-0001-6130-9579 0000-0003-1940-1990 0000-0003-4581-4967
    Data d'alta del registre: 2024-10-19
    Versió de l'article dipositat: info:eu-repo/semantics/acceptedVersion
    Enllaç font original: https://www.sciencedirect.com/science/article/abs/pii/S0022231318307579
    URL Document de llicència: https://repositori.urv.cat/ca/proteccio-de-dades/
    Referència a l'article segons font original: Journal Of Luminescence. 203 676-682
    Referència de l'ítem segons les normes APA: Zhang, Lizhen; Sun, Shijia; Lin, Zhoubin; Lin, Haifeng; Zhang, Ge; Mateos, Xavier; Maria Serres, Josep; Aguilo, Magdalena; Diaz, Francesc; Loiko, Pave (2018). Crystal growth, spectroscopy and first laser operation of a novel disordered tetragonal Tm:Na2La4(WO4)7tungstate crystal. Journal Of Luminescence, 203(), 676-682. DOI: 10.1016/j.jlumin.2018.07.016
    DOI de l'article: 10.1016/j.jlumin.2018.07.016
    Entitat: Universitat Rovira i Virgili
    Any de publicació de la revista: 2018
    Tipus de publicació: Journal Publications
  • Paraules clau:

    Atomic and Molecular Physics, and Optics,Biochemistry,Biophysics,Chemistry (Miscellaneous),Condensed Matter Physics,Optics
    Thulium ions
    Seven tungstates
    Luminescence
    Laser operation
    Judd-ofelt theory
    Absorption
    Química
    Optics
    Odontología
    Medicina ii
    Medicina i
    Materiais
    Interdisciplinar
    General chemistry
    Farmacia
    Ensino
    Engenharias iv
    Engenharias iii
    Engenharias ii
    Condensed matter physics
    Ciências biológicas ii
    Ciências biológicas i
    Ciências ambientais
    Ciência de alimentos
    Chemistry (miscellaneous)
    Chemistry (all)
    Biotecnología
    Biophysics
    Biochemistry
    Atomic and molecular physics, and optics
    Astronomia / física
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