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MoS2–Carbon Nanotube Hybrid Material Growth and Gas Sensing

  • Dades identificatives

    Identificador: imarina:9282670
    Autors:
    Deokar, GeetanjaliVancso, PeterArenal, RaulRavaux, FlorentCasanova-Chafer, JuanLlobet, EduardMakarova, AnnaVyalikh, DenisStruzzi, ClaudiaLambin, PhilippeJouiad, MustaphaColomer, Jean-Francois
    Resum:
    Hexagonal-shaped nanoplates (HNPs) of MoS2 on vertically aligned carbon nanotubes (CNTs) over a patterned area (a circular area of 1 cm2 diameter) are produced by chemical vapor deposition technique. With an optimized initial Mo film thickness, a uniform coverage of MoS2 HNPs with a thickness around 20 nm is achieved. The results confirm that the CNT template plays an important role in the MoS2 HNPs growth. Each MoS2 HNP consists of abundant exposed edges, interesting for sensing and catalysis applications. High crystallinity and quality of the as-produced material are revealed by X-ray photoelectron and Raman spectroscopies. Furthermore, NO2 gas-sensing studies show better sensitivity and recovery for MoS2/CNT samples as compared to pristine CNTs. The detection of NO2 gas in a few tens of parts per million to a few hundreds of parts per billion range, at room temperature, is achieved. Density-functional theory calculation indicates that the exposed edges of MoS2 play a significant role in the NO2 sensing as compared to horizontally aligned MoS2 layers. The present report can promote the research toward the fabrication of efficient and reliable MoS2-based hybrid materials for toxic gas-sensing applications for air quality monitoring in various environments. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
  • Altres:

    Autor segons l'article: Deokar, Geetanjali; Vancso, Peter; Arenal, Raul; Ravaux, Florent; Casanova-Chafer, Juan; Llobet, Eduard; Makarova, Anna; Vyalikh, Denis; Struzzi, Claudia; Lambin, Philippe; Jouiad, Mustapha; Colomer, Jean-Francois
    Departament: Enginyeria Electrònica, Elèctrica i Automàtica
    Autor/s de la URV: Casanova Chafer, Juan / Llobet Valero, Eduard
    Paraules clau: Nanoplates Mos2 Mos 2 Gas sensor Dft calculations Cnt
    Resum: Hexagonal-shaped nanoplates (HNPs) of MoS2 on vertically aligned carbon nanotubes (CNTs) over a patterned area (a circular area of 1 cm2 diameter) are produced by chemical vapor deposition technique. With an optimized initial Mo film thickness, a uniform coverage of MoS2 HNPs with a thickness around 20 nm is achieved. The results confirm that the CNT template plays an important role in the MoS2 HNPs growth. Each MoS2 HNP consists of abundant exposed edges, interesting for sensing and catalysis applications. High crystallinity and quality of the as-produced material are revealed by X-ray photoelectron and Raman spectroscopies. Furthermore, NO2 gas-sensing studies show better sensitivity and recovery for MoS2/CNT samples as compared to pristine CNTs. The detection of NO2 gas in a few tens of parts per million to a few hundreds of parts per billion range, at room temperature, is achieved. Density-functional theory calculation indicates that the exposed edges of MoS2 play a significant role in the NO2 sensing as compared to horizontally aligned MoS2 layers. The present report can promote the research toward the fabrication of efficient and reliable MoS2-based hybrid materials for toxic gas-sensing applications for air quality monitoring in various environments. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
    Àrees temàtiques: Química Mechanics of materials Mechanical engineering Materials science, multidisciplinary Materiais Interdisciplinar Chemistry, multidisciplinary Astronomia / física
    Accès a la llicència d'ús: https://creativecommons.org/licenses/by/3.0/es/
    Adreça de correu electrònic de l'autor: juan.casanova@urv.cat eduard.llobet@urv.cat
    Identificador de l'autor: 0000-0001-6164-4342
    Data d'alta del registre: 2024-10-12
    Versió de l'article dipositat: info:eu-repo/semantics/submittedVersion
    Enllaç font original: https://onlinelibrary.wiley.com/doi/10.1002/admi.201700801
    URL Document de llicència: https://repositori.urv.cat/ca/proteccio-de-dades/
    Referència a l'article segons font original: Advanced Materials Interfaces. 4 (24): 1700801-
    Referència de l'ítem segons les normes APA: Deokar, Geetanjali; Vancso, Peter; Arenal, Raul; Ravaux, Florent; Casanova-Chafer, Juan; Llobet, Eduard; Makarova, Anna; Vyalikh, Denis; Struzzi, Clau (2017). MoS2–Carbon Nanotube Hybrid Material Growth and Gas Sensing. Advanced Materials Interfaces, 4(24), 1700801-. DOI: 10.1002/admi.201700801
    DOI de l'article: 10.1002/admi.201700801
    Entitat: Universitat Rovira i Virgili
    Any de publicació de la revista: 2017
    Tipus de publicació: Journal Publications
  • Paraules clau:

    Chemistry, Multidisciplinary,Materials Science, Multidisciplinary,Mechanical Engineering,Mechanics of Materials
    Nanoplates
    Mos2
    Mos 2
    Gas sensor
    Dft calculations
    Cnt
    Química
    Mechanics of materials
    Mechanical engineering
    Materials science, multidisciplinary
    Materiais
    Interdisciplinar
    Chemistry, multidisciplinary
    Astronomia / física
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