Articles producció científica> Química Física i Inorgànica

Synthesis, spectroscopic characterization and laser operation of Ho3+in “mixed” (LuSc)2O3ceramics

  • Identification data

    Identifier: imarina:3996504
    Authors:
    Jing, WeiLoiko, PavelMaria Serres, JosepWang, YichengKifle, EsromVilejshikova, ElenaAguilo, MagdalenaDiaz, FrancescGriebner, UweHuang, HuiPetrov, ValentinMateos, Xavier
    Abstract:
    © 2018 Novel transparent Ho-doped sesquioxide ceramics are synthesized by high-temperature vacuum sintering and hot isostatic pressing. The spectroscopic properties of 1.4 at% and 3 at% Ho:(Lu,Sc)2O3ceramics are studied within Judd-Ofelt theory, yielding the intensity parameters Ω2= 7.863, Ω4= 1.843 and Ω6= 0.531 [10−20cm2]. The radiative lifetime of the5I7state is 10.63 ms. Absorption, stimulated-emission and gain cross-sections for the5I7→5I8Ho3+transition are calculated. At > 2 µm, the maximum σSE= 3.41× 10−21cm2at 2.101 µm. Under GaSb diode-pumping at 1.929 µm, the 1.4 at% Ho:(Lu,Sc)2O3ceramic laser generated 187 mW of quasi-continuous wave (CW) output at 2.114–2.135 µm with a slope efficiency η of 7.6%. When pumped at 1.946 µm with a Tm laser, η reached 25% while the CW output power was 20.5 mW. The Ho:(Lu,Sc)2O3ceramics are promising for broadband tunable and ultrashort pulse laser operation at ~ 2.1 µm.
  • Others:

    Author, as appears in the article.: Jing, Wei; Loiko, Pavel; Maria Serres, Josep; Wang, Yicheng; Kifle, Esrom; Vilejshikova, Elena; Aguilo, Magdalena; Diaz, Francesc; Griebner, Uwe; Huang, Hui; Petrov, Valentin; Mateos, Xavier
    Department: Química Física i Inorgànica
    URV's Author/s: Aguiló Díaz, Magdalena / Díaz Castrillón, Fernanda / Díaz González, Francisco Manuel / Mateos Ferré, Xavier / Serres Serres, Josep Maria
    Keywords: Transparent ceramics Spectroscopy Sesquioxides Laser operation Holmium
    Abstract: © 2018 Novel transparent Ho-doped sesquioxide ceramics are synthesized by high-temperature vacuum sintering and hot isostatic pressing. The spectroscopic properties of 1.4 at% and 3 at% Ho:(Lu,Sc)2O3ceramics are studied within Judd-Ofelt theory, yielding the intensity parameters Ω2= 7.863, Ω4= 1.843 and Ω6= 0.531 [10−20cm2]. The radiative lifetime of the5I7state is 10.63 ms. Absorption, stimulated-emission and gain cross-sections for the5I7→5I8Ho3+transition are calculated. At > 2 µm, the maximum σSE= 3.41× 10−21cm2at 2.101 µm. Under GaSb diode-pumping at 1.929 µm, the 1.4 at% Ho:(Lu,Sc)2O3ceramic laser generated 187 mW of quasi-continuous wave (CW) output at 2.114–2.135 µm with a slope efficiency η of 7.6%. When pumped at 1.946 µm with a Tm laser, η reached 25% while the CW output power was 20.5 mW. The Ho:(Lu,Sc)2O3ceramics are promising for broadband tunable and ultrashort pulse laser operation at ~ 2.1 µm.
    Thematic Areas: Química Optics Odontología Medicina ii Medicina i Materiais Interdisciplinar General chemistry Farmacia Ensino Engenharias iv Engenharias iii Engenharias ii Condensed matter physics Ciências biológicas ii Ciências biológicas i Ciências ambientais Ciência de alimentos Chemistry (miscellaneous) Chemistry (all) Biotecnología Biophysics Biochemistry Atomic and molecular physics, and optics Astronomia / física
    ISSN: 00222313
    Author's mail: josepmaria.serres@urv.cat fernanda.diaz@estudiants.urv.cat magdalena.aguilo@urv.cat xavier.mateos@urv.cat f.diaz@urv.cat
    Author identifier: 0000-0002-4299-538X 0000-0001-6130-9579 0000-0003-1940-1990 0000-0003-4581-4967
    Last page: 151
    Record's date: 2024-10-19
    Journal volume: 203
    Papper version: info:eu-repo/semantics/acceptedVersion
    Link to the original source: https://www.sciencedirect.com/science/article/abs/pii/S0022231318304757
    Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
    Papper original source: Journal Of Luminescence. 203 145-151
    APA: Jing, Wei; Loiko, Pavel; Maria Serres, Josep; Wang, Yicheng; Kifle, Esrom; Vilejshikova, Elena; Aguilo, Magdalena; Diaz, Francesc; Griebner, Uwe; Huan (2018). Synthesis, spectroscopic characterization and laser operation of Ho3+in “mixed” (LuSc)2O3ceramics. Journal Of Luminescence, 203(), 145-151. DOI: 10.1016/j.jlumin.2018.06.043
    Article's DOI: 10.1016/j.jlumin.2018.06.043
    Entity: Universitat Rovira i Virgili
    Journal publication year: 2018
    First page: 145
    Publication Type: Journal Publications
  • Keywords:

    Atomic and Molecular Physics, and Optics,Biochemistry,Biophysics,Chemistry (Miscellaneous),Condensed Matter Physics,Optics
    Transparent ceramics
    Spectroscopy
    Sesquioxides
    Laser operation
    Holmium
    Química
    Optics
    Odontología
    Medicina ii
    Medicina i
    Materiais
    Interdisciplinar
    General chemistry
    Farmacia
    Ensino
    Engenharias iv
    Engenharias iii
    Engenharias ii
    Condensed matter physics
    Ciências biológicas ii
    Ciências biológicas i
    Ciências ambientais
    Ciência de alimentos
    Chemistry (miscellaneous)
    Chemistry (all)
    Biotecnología
    Biophysics
    Biochemistry
    Atomic and molecular physics, and optics
    Astronomia / física
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