Author, as appears in the article.: Zhang, Lizhen; Loiko, Pavel; Maria Serres, Josep; Kifle, Esrom; Lin, Haifeng; Zhang, Ge; Vilejshikova, Elena; Dunina, Elena; Kornienko, Alexey; Fomicheva, Liudmila; Griebner, Uwe; Petrov, Valentin; Lin, Zhoubin; Chen, Weidong; Subbotin, Kirill; Aguilo, Magdalena; Diaz, Francesc; Mateos, Xavier
Department: Química Física i Inorgànica
URV's Author/s: Aguiló Díaz, Magdalena / Díaz González, Francisco Manuel / Mateos Ferré, Xavier / Serres Serres, Josep Maria
Keywords: Luminescence Laser operation Judd-ofelt theory Holmium ions Double tungstates
Abstract: © 2019 A monoclinic 0.86 at.% Ho3+:MgWO4 crystal is grown by the Top-Seeded-Solution Growth method. Its spectroscopic properties are studied with polarized light for E || a, b, c. The Ho3+ ion transition probabilities are determined within the modified Judd-Ofelt theory (mJ-O) accounting for the configuration interaction. The intensity parameters are Ω2 = 21.09, Ω4 = 4.42, Ω6 = 2.28 [10–20 cm2] and α = 0.053 [10-4 cm]. The calculated radiative lifetime of the 5I7 state is 6.18 ms. The Stark splitting of the 5I7 and 5I8 multiplets is determined with low-temperature spectroscopy. The absorption, stimulated-emission (SE) and gain cross-sections for the 5I8 ↔ 5I7 transition are derived. Ho3+:MgWO4 features a large Stark splitting of the ground-state (380 cm-1), high maximum σSE of 1.82 × 10–20 cm2 at 2.083 μm, broad gain spectra and high luminescence quantum yield making it suitable for efficient continuous-wave and mode-locked lasers at ∼2.1 μm. First laser operation of Ho3+:MgWO4 crystal is demonstrated at 2.104 μm reaching a slope efficiency of 72%.
Thematic Areas: Química Optics Odontología Medicina ii Medicina i Materiais Interdisciplinar General chemistry Farmacia Ensino Engenharias iv Engenharias iii Engenharias ii Condensed matter physics Ciências biológicas ii Ciências biológicas i Ciências ambientais Ciência de alimentos Chemistry (miscellaneous) Chemistry (all) Biotecnología Biophysics Biochemistry Atomic and molecular physics, and optics Astronomia / física
licence for use: https://creativecommons.org/licenses/by/3.0/es/
ISSN: 00222313
Author's mail: josepmaria.serres@urv.cat magdalena.aguilo@urv.cat xavier.mateos@urv.cat f.diaz@urv.cat
Author identifier: 0000-0002-4299-538X 0000-0001-6130-9579 0000-0003-1940-1990 0000-0003-4581-4967
Last page: 325
Record's date: 2024-10-19
Journal volume: 213
Papper version: info:eu-repo/semantics/acceptedVersion
Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
Papper original source: Journal Of Luminescence. 213 316-325
APA: Zhang, Lizhen; Loiko, Pavel; Maria Serres, Josep; Kifle, Esrom; Lin, Haifeng; Zhang, Ge; Vilejshikova, Elena; Dunina, Elena; Kornienko, Alexey; Fomich (2019). Growth, spectroscopy and first laser operation of monoclinic Ho3+:MgWO4 crystal. Journal Of Luminescence, 213(), 316-325. DOI: 10.1016/j.jlumin.2019.04.035
Entity: Universitat Rovira i Virgili
Journal publication year: 2019
First page: 316
Publication Type: Journal Publications
Repositori URV