Articles producció científica> Ciències Mèdiques Bàsiques

A fast algorithm for real-time monitoring of artificial radioisotopes in presence of variable natural radioactivity

  • Identification data

    Identifier: imarina:9296463
    Authors:
    Cerezo, ACerezo, APrieto, EPrieto, EReichardt, IReichardt, ICasanovas, RCasanovas, RSalvado, MSalvado, M
    Abstract:
    We present an agile, hardware independent analysis methodology based on the spectral windows technique to detect and quantify the environmental activity concentration of artificial isotopes of interest. The method removes counts from Compton scattering, peak overlapping, intrinsic background and other unconsidered contributions to the spectral region where photopeaks from artificial elements are expected. Taking into account the varying concentration of 214Bi, 214Pb, and 212Pb, we compute the activity concentration of the artificial isotopes (when detectable), or a variable Minimum Detectable Activity Concentration (MDAC). This allows to set statistically robust early-warning levels. In the scenario with the lowest concentration of natural occurring isotopes, and for 10-min integration time, we achieve a MDAC of 5.4/4.1/3.9 (Bq/m³) for 131I/137Cs/60Co using a LaBr3(Ce) detector; and 4.2/2.8/2.7 (Bq/m³) for 131I/137Cs/60Co with a SrI2(Eu) detector.
  • Others:

    Author, as appears in the article.: Cerezo, A; Cerezo, A; Prieto, E; Prieto, E; Reichardt, I; Reichardt, I; Casanovas, R; Casanovas, R; Salvado, M; Salvado, M
    Department: Ciències Mèdiques Bàsiques
    URV's Author/s: Casanovas Alegre, Ramon / Cerezo Fernández, Agustín / Salvadó Artells, Marçal
    Keywords: Sri (eu) 2 Scintillation gamma-ray spectrometry Scintillation gamma -ray spectrometry Natural isotope Labr (ce) 3 Gamma-ray spectrometry Environmental surveillance network Early warning sri2(eu) natural isotope nai(tl) labr 3 (ce) environmental surveillance network early warning code calibration
    Abstract: We present an agile, hardware independent analysis methodology based on the spectral windows technique to detect and quantify the environmental activity concentration of artificial isotopes of interest. The method removes counts from Compton scattering, peak overlapping, intrinsic background and other unconsidered contributions to the spectral region where photopeaks from artificial elements are expected. Taking into account the varying concentration of 214Bi, 214Pb, and 212Pb, we compute the activity concentration of the artificial isotopes (when detectable), or a variable Minimum Detectable Activity Concentration (MDAC). This allows to set statistically robust early-warning levels. In the scenario with the lowest concentration of natural occurring isotopes, and for 10-min integration time, we achieve a MDAC of 5.4/4.1/3.9 (Bq/m³) for 131I/137Cs/60Co using a LaBr3(Ce) detector; and 4.2/2.8/2.7 (Bq/m³) for 131I/137Cs/60Co with a SrI2(Eu) detector.
    Thematic Areas: Zootecnia / recursos pesqueiros Saúde coletiva Radiation Química Physics, atomic, molecular & chemical Odontología Nutrição Nuclear science & technology Medicina veterinaria Medicina ii Medicina i Materiais Interdisciplinar Geografía Geociências Farmacia Ensino Engenharias iv Engenharias iii Engenharias ii Engenharias i Ciências biológicas iii Ciências biológicas ii Ciências biológicas i Ciências ambientais Ciências agrárias i Ciência de alimentos Chemistry, physical Biotecnología Biodiversidade Astronomia / física Antropologia / arqueologia
    licence for use: https://creativecommons.org/licenses/by/3.0/es/
    Author's mail: ramon.casanovas@urv.cat agustin.cerezo@urv.cat agustin.cerezo@urv.cat m.salvado@urv.cat
    Author identifier: 0000-0002-3954-158X 0000-0002-9399-6649
    Record's date: 2024-09-28
    Papper version: info:eu-repo/semantics/publishedVersion
    Link to the original source: https://www.sciencedirect.com/science/article/abs/pii/S0969806X23001913
    Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
    Papper original source: Radiation Physics And Chemistry. 209 110946-
    APA: Cerezo, A; Cerezo, A; Prieto, E; Prieto, E; Reichardt, I; Reichardt, I; Casanovas, R; Casanovas, R; Salvado, M; Salvado, M (2023). A fast algorithm for real-time monitoring of artificial radioisotopes in presence of variable natural radioactivity. Radiation Physics And Chemistry, 209(), 110946-. DOI: 10.1016/j.radphyschem.2023.110946
    Article's DOI: 10.1016/j.radphyschem.2023.110946
    Entity: Universitat Rovira i Virgili
    Journal publication year: 2023
    Publication Type: Journal Publications
  • Keywords:

    Chemistry, Physical,Nuclear Science & Technology,Physics, Atomic, Molecular & Chemical,Radiation
    Sri (eu) 2
    Scintillation gamma-ray spectrometry
    Scintillation gamma -ray spectrometry
    Natural isotope
    Labr (ce) 3
    Gamma-ray spectrometry
    Environmental surveillance network
    Early warning
    sri2(eu)
    natural isotope
    nai(tl)
    labr 3 (ce)
    environmental surveillance network
    early warning
    code
    calibration
    Zootecnia / recursos pesqueiros
    Saúde coletiva
    Radiation
    Química
    Physics, atomic, molecular & chemical
    Odontología
    Nutrição
    Nuclear science & technology
    Medicina veterinaria
    Medicina ii
    Medicina i
    Materiais
    Interdisciplinar
    Geografía
    Geociências
    Farmacia
    Ensino
    Engenharias iv
    Engenharias iii
    Engenharias ii
    Engenharias i
    Ciências biológicas iii
    Ciências biológicas ii
    Ciências biológicas i
    Ciências ambientais
    Ciências agrárias i
    Ciência de alimentos
    Chemistry, physical
    Biotecnología
    Biodiversidade
    Astronomia / física
    Antropologia / arqueologia
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