Articles producció científica> Enginyeria Química

Computational Fluid Dynamic study of gas mixtures in a Non-Thermal Plasma reactor for CO2 conversion

  • Identification data

    Identifier: imarina:9405937
    Authors:
    Mas-Peiro, CristinaFerret, Felix LlovellIbar, Oriol Pou
    Abstract:
    CO2 utilization has been an emerging technology of increasing global interest due to its direct impact in limiting greenhouse gas emissions. In this contribution, the fluid dynamic behavior of a CO2 conversion nonthermal plasma (NTP) in a dielectric barrier discharge (DBD) reactor is studied through computational fluid dynamics (CFD) simulations. Calculations are provided in conjunction with experimental results and the thermodynamic characterization of the compounds and mixtures involved. This CFD study utilizes a well -established methodology that allows the optimization of fluid flow with limited computational burden. Firstly, results are presented for an Example Case, in which several variables are studied both at the final iteration as well as across iterations. Secondly, a range of Study Cases, changing the inlet composition and volume rate, are presented. Average velocity is one of the most significant variables to predict the reactor's yield, while the temperature, density and pressure in the reactor remain, in most cases, almost constant. The resulting CFD computations describe the behavior of the fluids in the reactor in a predictive manner for future experimental results. Limitations in the fluid's characterization occur due to not explicitly including the plasma reaction, which will be aimed at in future contributions.
  • Others:

    Author, as appears in the article.: Mas-Peiro, Cristina; Ferret, Felix Llovell; Ibar, Oriol Pou
    Department: Enginyeria Química
    URV's Author/s: Llovell Ferret, Fèlix Lluís
    Keywords: Co2 conversion Computational fluid dynamics Dielectric barrier discharge plasma Fluid mechanics Non-thermal plasma Plasma reacto
    Abstract: CO2 utilization has been an emerging technology of increasing global interest due to its direct impact in limiting greenhouse gas emissions. In this contribution, the fluid dynamic behavior of a CO2 conversion nonthermal plasma (NTP) in a dielectric barrier discharge (DBD) reactor is studied through computational fluid dynamics (CFD) simulations. Calculations are provided in conjunction with experimental results and the thermodynamic characterization of the compounds and mixtures involved. This CFD study utilizes a well -established methodology that allows the optimization of fluid flow with limited computational burden. Firstly, results are presented for an Example Case, in which several variables are studied both at the final iteration as well as across iterations. Secondly, a range of Study Cases, changing the inlet composition and volume rate, are presented. Average velocity is one of the most significant variables to predict the reactor's yield, while the temperature, density and pressure in the reactor remain, in most cases, almost constant. The resulting CFD computations describe the behavior of the fluids in the reactor in a predictive manner for future experimental results. Limitations in the fluid's characterization occur due to not explicitly including the plasma reaction, which will be aimed at in future contributions.
    Thematic Areas: Chemical engineering (all) Chemical engineering (miscellaneous) Chemistry Chemistry (all) Chemistry (miscellaneous) Chemistry, multidisciplinary Ciência de alimentos Ciências biológicas i Engenharias i Engenharias ii Engenharias iii General chemical engineering General chemistry Interdisciplinar Química
    licence for use: https://creativecommons.org/licenses/by/3.0/es/
    Author's mail: felix.llovell@urv.cat
    Author identifier: 0000-0001-7109-6810
    Record's date: 2024-12-14
    Papper version: info:eu-repo/semantics/publishedVersion
    Papper original source: Afinidad. 81 (601): 57-67
    APA: Mas-Peiro, Cristina; Ferret, Felix Llovell; Ibar, Oriol Pou (2024). Computational Fluid Dynamic study of gas mixtures in a Non-Thermal Plasma reactor for CO2 conversion. Afinidad, 81(601), 57-67. DOI: 10.55815/424061
    Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
    Entity: Universitat Rovira i Virgili
    Journal publication year: 2024
    Publication Type: Journal Publications
  • Keywords:

    Chemical Engineering (Miscellaneous),Chemistry,Chemistry (Miscellaneous),Chemistry, Multidisciplinary
    Co2 conversion
    Computational fluid dynamics
    Dielectric barrier discharge plasma
    Fluid mechanics
    Non-thermal plasma
    Plasma reacto
    Chemical engineering (all)
    Chemical engineering (miscellaneous)
    Chemistry
    Chemistry (all)
    Chemistry (miscellaneous)
    Chemistry, multidisciplinary
    Ciência de alimentos
    Ciências biológicas i
    Engenharias i
    Engenharias ii
    Engenharias iii
    General chemical engineering
    General chemistry
    Interdisciplinar
    Química
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