Articles producció científica> Química Física i Inorgànica

The multi-faceted mechano-bactericidal mechanism of nanostructured surfaces

  • Datos identificativos

    Identificador: imarina:6381275
    Handle: http://hdl.handle.net/20.500.11797/imarina6381275
  • Autores:

    Ivanova EP, Linklater DP, Werner M, Baulin VA, Xu X, Vrancken N, Rubanov S, Hanssen E, Wandiyanto J, Truong VK, Elbourne A, Maclaughlin S, Juodkazis S, Crawford RJ
  • Otros:

    Autor según el artículo: Ivanova EP, Linklater DP, Werner M, Baulin VA, Xu X, Vrancken N, Rubanov S, Hanssen E, Wandiyanto J, Truong VK, Elbourne A, Maclaughlin S, Juodkazis S, Crawford RJ
    Departamento: Química Física i Inorgànica
    Autor/es de la URV: Baulin, Vladimir
    Palabras clave: Younǵs modulus Staphylococcus-aureus Natural nanotopography Nanostructured surface Mechano-bactericidal Infectious-diseases-society Gecko skin Force Black silicon Attachment Antibacterial Adhesion
    Resumen: The mechano-bactericidal activity of nanostructured surfaces has become the focus of intensive research toward the development of a new generation of antibacterial surfaces, particularly in the current era of emerging antibiotic resistance. This work demonstrates the effects of an incremental increase of nanopillar height on nanostructure-induced bacterial cell death. We propose that the mechanical lysis of bacterial cells can be influenced by the degree of elasticity and clustering of highly ordered silicon nanopillar arrays. Herein, silicon nanopillar arrays with diameter 35 nm, periodicity 90 nm and increasing heights of 220, 360, and 420 nm were fabricated using deep UV immersion lithography. Nanoarrays of 360-nm-height pillars exhibited the highest degree of bactericidal activity toward both Gram stain-negative Pseudomonas aeruginosa and Gram stain-positive Staphylococcus aureus bacteria, inducing 95 ± 5% and 83 ± 12% cell death, respectively. At heights of 360 nm, increased nanopillar elasticity contributes to the onset of pillar deformation in response to bacterial adhesion to the surface. Theoretical analyses of pillar elasticity confirm that deflection, deformation force, and mechanical energies are more significant for the substrata possessing more flexible pillars. Increased storage and release of mechanical energy may explain the enhanced bactericidal action of these nanopillar arrays toward bacterial cells contacting the surface; however, with further increase of nanopillar height (420 nm), the forces (and tensions) can be partially compensated by irreversible interpillar adhesion that reduces their bactericidal effect. These findings can be used to inform the design of next-generation mechano-responsive surfaces with tuneable bactericidal characteristics for antimicrobial surface technologies.
    Áreas temáticas: Zootecnia / recursos pesqueiros Saúde coletiva Química Psicología Odontología Multidisciplinary sciences Multidisciplinary Medicina veterinaria Medicina iii Medicina ii Medicina i Matemática / probabilidade e estatística Interdisciplinar Geografía Geociências General o multidisciplinar Farmacia Engenharias iv Engenharias iii Engenharias ii Engenharias i Educação física Ciencias sociales Ciências biológicas iii Ciências biológicas ii Ciências biológicas i Ciências ambientais Ciências agrárias i Ciência da computação Biotecnología Biodiversidade Astronomia / física Antropologia / arqueologia Anthropology
    Acceso a la licencia de uso: https://creativecommons.org/licenses/by/3.0/es/
    ISSN: 00278424
    Direcció de correo del autor: vladimir.baulin@urv.cat
    Identificador del autor: 0000-0003-2086-4271
    Fecha de alta del registro: 2023-02-22
    Versión del articulo depositado: info:eu-repo/semantics/publishedVersion
    Enlace a la fuente original: https://www.pnas.org/content/117/23/12598
    URL Documento de licencia: http://repositori.urv.cat/ca/proteccio-de-dades/
    Referencia al articulo segun fuente origial: Proceedings Of The National Academy Of Sciences Of The United States Of America. 117 (23): 12598-12605
    Referencia de l'ítem segons les normes APA: Ivanova EP, Linklater DP, Werner M, Baulin VA, Xu X, Vrancken N, Rubanov S, Hanssen E, Wandiyanto J, Truong VK, Elbourne A, Maclaughlin S, Juodkazis S (2020). The multi-faceted mechano-bactericidal mechanism of nanostructured surfaces. Proceedings Of The National Academy Of Sciences Of The United States Of America, 117(23), 12598-12605. DOI: 10.1073/pnas.1916680117
    DOI del artículo: 10.1073/pnas.1916680117
    Entidad: Universitat Rovira i Virgili
    Año de publicación de la revista: 2020
    Tipo de publicación: Journal Publications
  • Palabras clave:

    Multidisciplinary,Multidisciplinary Sciences
    Younǵs modulus
    Staphylococcus-aureus
    Natural nanotopography
    Nanostructured surface
    Mechano-bactericidal
    Infectious-diseases-society
    Gecko skin
    Force
    Black silicon
    Attachment
    Antibacterial
    Adhesion
    Zootecnia / recursos pesqueiros
    Saúde coletiva
    Química
    Psicología
    Odontología
    Multidisciplinary sciences
    Multidisciplinary
    Medicina veterinaria
    Medicina iii
    Medicina ii
    Medicina i
    Matemática / probabilidade e estatística
    Interdisciplinar
    Geografía
    Geociências
    General o multidisciplinar
    Farmacia
    Engenharias iv
    Engenharias iii
    Engenharias ii
    Engenharias i
    Educação física
    Ciencias sociales
    Ciências biológicas iii
    Ciências biológicas ii
    Ciências biológicas i
    Ciências ambientais
    Ciências agrárias i
    Ciência da computação
    Biotecnología
    Biodiversidade
    Astronomia / física
    Antropologia / arqueologia
    Anthropology
  • Documentos:

  • Cerca a google

    Search to google scholar