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Disordered Tm:Ca9La(VO4)7: A novel crystal with potential for broadband tunable lasing

  • Identification data

    Identifier: PC:2576
    Handle: https://hdl.handle.net/20.500.11797/PC2576
    Authors:
    X. MATEOSZ. ZHANGP. LOIKOH. WUJ. M. SERRESH. F. LINW. D. CHENG. ZHANGL. Z. ZHANGV. PETROVF. DÍAZM. AGUILÓU. GRIEBNERY. C. WANGE. VILEJSHIKOVAK. YUMASHEVZ. B. LIN
    Abstract:
    We report on the crystal growth, structural and spectroscopic investigation of a novel trigonal calcium vanadate crystal, Tm3+:Ca9La(VO4)7. Polarized absorption, stimulatedemission and gain cross-section spectra are determined for this material. The maximum ¿SE corresponding to the 3F4 ¿ 3H6 transition amounts to 1.28 × 10-20 cm2 at 1854 nm for ¿- polarization. The measured lifetime of the Tm3+ ions in the 3F4 state is 1.19 ms. The Judd- Ofelt analysis performed yielded intensity parameters of ¿2 = 4.682, ¿4 = 0.659 and ¿6 = 0.475 [10-20 cm2]. The polarized Raman spectra indicate a strong and broad band centered at 867 cm-1. Owing to the disordered nature of Ca9La(VO4)7, the Tm3+ ions exhibit a broad and smooth gain profile at ~2 ¿m. The spectroscopic properties of Tm3+:Ca9La(VO4)7 are very promising for broadly tunable and ultrashort pulse lasers near 2 ¿m.

  • Others:

    Author, as appears in the article.: X. MATEOS; Z. ZHANG; P. LOIKO; H. WU; J. M. SERRES; H. F. LIN; W. D. CHEN; G. ZHANG; L. Z. ZHANG; V. PETROV; F. DÍAZ; M. AGUILÓ; U. GRIEBNER; Y. C. WANG; E. VILEJSHIKOVA; K. YUMASHEV; Z. B. LIN
    Department: Química Física i Inorgànica
    URV's Author/s: MATEOS FERRÉ, XAVIER; Z. ZHANG; P. LOIKO; H. WU; J. M. SERRES; H. F. LIN; W. D. CHEN; G. ZHANG; L. Z. ZHANG; V. PETROV; DÍAZ GONZÁLEZ, FRANCISCO MANUEL; AGUILÓ DÍAZ, MAGDALENA; U. GRIEBNER; Y. C. WANG; E. VILEJSHIKOVA; K. YUMASHEV; Z. B. LIN
    Keywords: Ultrashort pulses Tunable lasing Calcium
    Abstract: We report on the crystal growth, structural and spectroscopic investigation of a novel trigonal calcium vanadate crystal, Tm3+:Ca9La(VO4)7. Polarized absorption, stimulatedemission and gain cross-section spectra are determined for this material. The maximum ¿SE corresponding to the 3F4 ¿ 3H6 transition amounts to 1.28 × 10-20 cm2 at 1854 nm for ¿- polarization. The measured lifetime of the Tm3+ ions in the 3F4 state is 1.19 ms. The Judd- Ofelt analysis performed yielded intensity parameters of ¿2 = 4.682, ¿4 = 0.659 and ¿6 = 0.475 [10-20 cm2]. The polarized Raman spectra indicate a strong and broad band centered at 867 cm-1. Owing to the disordered nature of Ca9La(VO4)7, the Tm3+ ions exhibit a broad and smooth gain profile at ~2 ¿m. The spectroscopic properties of Tm3+:Ca9La(VO4)7 are very promising for broadly tunable and ultrashort pulse lasers near 2 ¿m.
    Research group: Física i Cristal.lografia de Materials Física i Cristal·lografia de Nanomaterials
    Thematic Areas: Química Química Chemistry
    licence for use: https://creativecommons.org/licenses/by/3.0/es/
    ISSN: 2159-3930
    Author identifier: 0000-0003-1940-1990; n/a; 0000-0002-4270-0668; n/a; 0000-0002-4299-538X; n/a; n/a; n/a; n/a; n/a; 0000-0003-4581-4967; 0000-0001-6130-9579; n/a; n/a; n/a; n/a; n/a
    Record's date: 2017-02-23
    Last page: 493
    Journal volume: 7
    Papper version: info:eu-repo/semantics/publishedVersion
    Licence document URL: https://repositori.urv.cat/ca/proteccio-de-dades/
    Entity: Universitat Rovira i Virgili
    Journal publication year: 2017
    First page: 484
    Publication Type: Article Artículo Article

  • Keywords:

    Calci
    Làsers sintonitzables
    Ultrashort pulses
    Tunable lasing
    Calcium
    Química
    Química
    Chemistry
    2159-3930

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